@article {2572,
	title = {Fate of terrigenous organic matter across the Laptev Sea from the mouth of the Lena River to the deep sea of the Arctic interior},
	journal = {Biogeosciences},
	volume = {13},
	year = {2016},
	month = {Jan-01-2016},
	pages = {5003 - 5019},
	abstract = {Ongoing global warming in high latitudes may cause an increasing supply of permafrost-derived organic carbon through both river discharge and coastal erosion to the Arctic shelves. Mobilized permafrost carbon can be either buried in sediments, transported to the deep sea or degraded to CO2 and outgassed, potentially constituting a positive feedback to climate change.

This study aims to assess the fate of terrigenous organic carbon (TerrOC) in the Arctic marine environment by exploring how it changes in concentration, composition and degradation status across the wide Laptev Sea shelf. We analyzed a suite of terrestrial biomarkers as well as source-diagnostic bulk carbon isotopes (δ13C, Δ14C) in surface sediments from a Laptev Sea transect spanning more than 800 km from the Lena River mouth (< 10 m water depth) across the shelf to the slope and rise (2000{\textendash}3000 m water depth). These data provide a broad view on different TerrOC pools and their behavior during cross-shelf transport. The concentrations of lignin phenols, cutin acids and high-molecular-weight (HMW) wax lipids (tracers of vascular plants) decrease by 89{\textendash}99 \% along the transect. Molecular-based degradation proxies for TerrOC (e.g., the carbon preference index of HMW lipids, the HMW acids / alkanes ratio and the acid / aldehyde ratio of lignin phenols) display a trend to more degraded TerrOC with increasing distance from the coast. We infer that the degree of degradation of permafrost-derived TerrOC is a function of the time spent under oxic conditions during protracted cross-shelf transport. Future work should therefore seek to constrain cross-shelf transport times in order to compute a TerrOC degradation rate and thereby help to quantify potential carbon{\textendash}climate feedbacks.},
	doi = {10.5194/bg-13-5003-201610.5194/bg-13-5003-2016},
	url = {http://www.biogeosciences.net/13/5003/2016},
	author = {Broder, Lisa and Tesi, Tommaso and Salvad?, Joan A. and Semiletov, Igor P. and Dudarev, Oleg V. and Gustafsson, ?rjan}
}
@article {2573,
	title = {Historical records of organic matter supply and degradation status in the East Siberian Sea},
	journal = {Organic Geochemistry},
	volume = {91},
	year = {2016},
	month = {Jan-01-2016},
	pages = {16 - 30},
	abstract = {Destabilization and degradation of permafrost carbon in the Arctic regions could constitute a positive feedback to climate change. A better understanding of its fate upon discharge to the Arctic shelf is therefore needed. In this study, bulk carbon isotopes as well as terrigenous and marine biomarkers were used to construct two centennial records in the East Siberian Sea. Differences in topsoil and Pleistocene Ice Complex Deposit permafrost concentrations, modeled using δ13C and Δ14C, were larger between inner and outer shelf than the changes over time. Similarly, lignin-derived phenol and cutin acid concentrations differed by a factor of ten between the two stations, but did not change significantly over time, consistent with the dual-carbon isotope model. High molecular weight (HMW) n-alkane and n-alkanoic acid concentrations displayed a smaller difference between the two stations (factor of 3{\textendash}6). By contrast, the fraction for marine OC drastically decreased during burial with a half-life of 19{\textendash}27 years. Vegetation and degradation proxies suggested supply of highly degraded gymnosperm wood tissues. Lipid Carbon Preference Index (CPI) values indicated more extensively degraded HMW n-alkanes on the outer shelf with no change over time, whereas n-alkanoic acids appeared to be less degraded toward the core top with no large differences between the stations. Taken together, our results show larger across-shelf changes than down-core trends. Further investigation is required to establish whether the observed spatial differences are due to different sources for the two depositional settings or, alternatively, a consequence of hydrodynamic sorting combined with selective degradation during cross-shelf transport.},
	keywords = {210Pb, Arctic, East Siberian Arctic Shelf, HMW wax lipids, Lignin, Monte Carlo, δ13C, Δ14C},
	issn = {01466380},
	doi = {10.1016/j.orggeochem.2015.10.008},
	url = {https://doi.org/10.1016/j.orggeochem.2015.10.008},
	author = {Broder, Lisa and Tesi, Tommaso and Andersson, August and Eglinton, Timothy I. and Semiletov, Igor P. and Dudarev, Oleg V. and Roos, Per and Gustafsson, ?rjan}
}
